Information About

Tetrairidium Dodecacarbonyl




  IUPACName Tetrairidium dodecacarbonyl
  OtherNames iridium(0) carbonyl iridium carbonyl iridium dodecacarbonyl
  Section1 {{Chembox Identifiers
  CASNo 18827-81-1


  Section2 {{Chembox Properties
  Formula C<sub>12</sub>O<sub>12</sub>Ir<sub>4</sub>
  MolarMass 110492 g/mol
  Appearance Canary-yellow crystals
  MeltingPt 195 °C
  SolubleOther Chlorocarbon s, Toluene , Tetrahydrofuran


  Section3 {{Chembox Hazards


  Section8 {{Chembox Related
  OtherCpds Tetrarhodium Dodecacarbonyl




Tetrairidium dodecacarbonyl is the Chemical Compound with the Formula Ir4(CO)12. This tetrahedral Cluster is the most common and most stable "binary" Carbonyl of Iridium . This air-stable species is only poorly soluble in organic solvents. It has been used to prepare bimetallic clusters and catalysts, e.g. for the Water Gas Shift Reaction , and reforming, but these studies are of purely academic interest.


STRUCTURE

Each Ir center is octahedral, being bonded to 3 other iridium atoms and three CO ligands. Ir4(CO)12 has Td Symmetry . The related clusters Rh4(CO)12 and Co4(CO)12 have C3v symmetry because of the presence of three bridging CO ligands in each.


PREPARATION

It is prepared in two steps by reductive carbonylation of hydrated Iridium Trichloride . The first step give {Link without Title} -.Pergola, R. D.; Garlaschelli, L.; Matinengo, S. "Dodecacarbonyltetrairidium: Ir4(CO)12" Inorganic Syntheses, 1990, volume 28, pp. 245-247. ISBN 0-471-52619-3
:IrCl3 + 3 CO + H2O → {Link without Title} - + HCl- + CO2 + H+
:4 {Link without Title} - + 6 CO + 2 H2O → Ir4(CO)12 + 2 CO2 + 4 H+ + 8 Cl-


REFERENCES


http://www.webelements.com/webelements/compounds/text/Ir/C12Ir4O12-18827811.html
http://arjournals.annualreviews.org/